non-thermal

This data set contains the data shown in the corresponding publication in Plasma Sources Science and Technology (https://doi.org/10.1088/1361-6595/acb815). This publication presents the first implementation of terahertz (THz) quantum cascade lasers (QCLs) for high-resolution absorption spectroscopy on plasmas. Absolute densities of ground state atomic oxygen were directly obtained by using the fine structure transition at approximately 4.75 THz.

A self-consistent fluid model has been successfully developed and employed to model an electron cyclotron resonance driven hydrogen plasma at low pressure. This model has enabled key insights to be made on the mutual interaction of microwave propagation, power density, plasma generation, and species transport at conditions where the critical plasma density is exceeded. The model has been verified by two experimental methods.

A study on the scalability of discharge characteristics of a single-filament dielectric barrier discharge (DBD) to a spatially one-dimensional multi-filament arrangement driven by the same high-voltage (HV) pulses was performed for a gas mixture of 0.1 vol% O2 in N2 at 1 bar. Both arrangements feature a 1 mm gap with dielectric-covered electrodes featuring two hemispherical alumina caps for the single-filament and two parallel alumina-tubes for the multi-filament arrangement.

Modelling results obtained using an extended reaction kinetics model (RKM) suitable for the analysis of weakly ionised, non-thermal argon plasmas with gas temperatures around 300K at sub-atmospheric and atmospheric pressures are presented. Modelling was performed by means of a time- and space-dependent fluid model for two different dielectric barrier discharge configurations as well as for a micro-scaled atmospheric-pressure plasma jet setup. The results are also compared with measurements, as well as with modelling data obtained by use of a previously established 15-species RKM.

Presented data was obtained from the analysis of the impact of the electrode proximity on the streamer breakdown and development of pulsed-driven dielectric barrier discharges (DBDs) in a singlefilament arrangement in a gas mixture of 0.1 vol% O2 in N2 at 0.6 bar and 1.0 bar. The gap distance was varied from 0.5 mm to 1.5 mm, and the applied voltage was adapted correspondingly to create comparable breakdown conditions in the gap. Fast electrical measurements provided insight into discharge characteristics such as the transferred charge and consumed energy.

The results of the modelling of an atmospheric-pressure dielectric barrier discharge (DBD) in argon obtained using a time-dependent and spatially two-dimensional fluid-Poisson model in axisymmetric geometry are provided in this dataset.

Absolute ground state atomic hydrogen densities were measured, by utilisation of two-photon absorption laser induced fluorescence (TALIF), in a low pressure electron cyclotron resonance plasma as a function of nitrogen admixtures - 0 to 5000 ppm. At nitrogen admixtures of 1500 ppm and higher the spectral distribution of the fluorescence changes from a single Gaussian to a double Gaussian distribution; this is due to a separate, nascent, contribution arising from the photolysis of an ammonia molecule.

The data set comprises full cavity ring-down spectra and absorption coefficients obtained from on-off-resonance measurements, in order to determine the spatial distribution of HO₂ in the cold atmospheric pressure plasma jet kINPen-sci. Therefore, the plasma jet was operated with 3 slm Ar and 3000 ppm water, and was equipped with a gas curtain of 5 slm O₂. To determine the effective absorption length, the HO₂ absorption was measured in radial direction. These radial fits had a Gaussian-like shape.